Unprecedented redox-driven ligand ejection in nickel(II)-diiminosemiquinonate radical complexes.

Nickel(II) complexes of (M:L) stoichiometries 1:1 (1) and 1:2 (2) were prepd. from a polydentate ligand involving diiminosemiquinonate radicals. Both were characterized by x-ray diffraction, visible-NIR and EPR spectroscopy as well as electrochem. Ligand-centered oxidn. of 1 promotes ligand ejection to give 2. [on SciFinder(R)]

Références

Titre
Unprecedented redox-driven ligand ejection in nickel(II)-diiminosemiquinonate radical complexes.
Type de publication
Article de revue
Année de publication
2014
Revue
Chem. Commun. (Cambridge, United Kingdom)
Volume
50
Pagination
1918–1920
ISSN
1359-7345
Soumis le 12 avril 2018