Structural snapshots of the rearrangement of the bis(di-tert-butyl-aminophenyl)amine pincer ligand in the presence of transition metal ions

The bis(di-tert-butyl-aminophenyl)amine ligand H3LN{,}N{,}N was reacted with Mn(ii){,} Co(ii){,} Fe(iii) and Cu(ii) salts in air. The ligand undergoes oxidative transformations{,} which involve intra and intermolecular C–N and N–N bond formations. A rare aromatic C–N bond cleavage leading to a C–O bond has also been observed.

Références

Titre
Structural snapshots of the rearrangement of the bis(di-tert-butyl-aminophenyl)amine pincer ligand in the presence of transition metal ions
Type de publication
Article de revue
Année de publication
2018
Revue
Dalton Trans.
Volume
47
Pagination
11303-11307
Soumis le 28 août 2018